Stretchable ITO-Free Organic Solar Cells with Intrinsic Anti-Reflection Substrate for High-Efficiency Outdoor and Indoor Energy Harvesting

Jiaming Huang, Zhiwei Ren, Yaokang Zhang, Kuan Liu, Hengkai Zhang, Hua Tang, Cenqi Yan, Zijian Zheng, Gang Li

Research output: Journal article publicationJournal articleAcademic researchpeer-review

5 Citations (Scopus)

Abstract

Flexible photovoltaic devices are promising candidates for triggering the Internet of Things (IoT). However, the power conversion efficiencies (PCEs) of flexible organic photovoltaic (OPV) devices with high conductivity poly(3,4-ethylene dioxythiophene):polystyrene sulfonate (PEDOT:PSS) electrodes on plastic are lagging behind the rigid devices due to the low transmittance of polyethylene terephthalate (PET)/PEDOT:PSS. Moreover, the poor stretchability of the commonly used plastic substrates largely hinders the practical application of wearable devices. Herein, a novel stretchable indium tin oxide (ITO)-free OPV device with a surface-texturing polydimethylsiloxane (PDMS) substrate for outdoor strong- and indoor dim-light energy harvesting is reported. The high diffuse transmittance and haze effect of the substrate enable stretchable ITO-free devices, yielding a high PCE of 15.3% under 1 sun illumination. More excitingly, the stretchable device based on textured PDMS/PEDOT:PSS maintains a comparable PCE of 20.5% (20.8% for the rigid device) under indoor light illumination. Notably, the stretchable device is much more insensitive to the light direction, maintaining 38.5% of the initial PCE at an extremely small incident angle of 10° (16.3% for glass/ITO-based counterpart). The texturing stretchable substrate provides a new direction for achieving high performance and enhanced light utilization for the stretchable light-harvesting device, suitable for indoor and outdoor applications.

Original languageEnglish
Article number2010172
JournalAdvanced Functional Materials
Volume31
Issue number16
DOIs
Publication statusPublished - 15 Apr 2021

Keywords

  • anti-reflection
  • indoor applications, ITO-free
  • outdoor applications
  • stretchable photovoltaic electronics
  • texturing stretchable substrates

ASJC Scopus subject areas

  • Chemistry(all)
  • Materials Science(all)
  • Condensed Matter Physics

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