Room-temperature processed tin oxide thin film as effective hole blocking layer for planar perovskite solar cells

Hong Tao, Zhibin Ma, Guang Yang, Haoning Wang, Hao Long, Hongyang Zhao, Pingli Qin, Guojia Fang

Research output: Journal article publicationJournal articleAcademic researchpeer-review

50 Citations (Scopus)

Abstract

Tin oxide (SnO 2 ) film with high mobility and good transmittance has been reported as a promising semiconductor material for high performance perovskite solar cells (PSCs). In this study, ultrathin SnO 2 film synthesized by radio frequency magnetron sputtering (RFMS) method at room temperature was employed as hole blocking layer for planar PSCs. The room-temperature sputtered SnO 2 film not only shows favourable energy band structure but also improves the surface topography of fluorine doped SnO 2 (FTO) substrate and perovskite (CH 3 NH 3 PbI 3 ) layer. Thus, this SnO 2 hole blocking layer can efficiently promote electron transport and suppress carrier recombination. Furthermore, the best efficiency of 13.68% was obtained for planar PSC with SnO 2 hole blocking layer prepared at room temperature. This research highlights the room-temperature preparation process of hole blocking layer in PSC and has a certain reference significance for the usage of flexible and low-cost substrates.

Original languageEnglish
Pages (from-to)1336-1343
Number of pages8
JournalApplied Surface Science
Volume434
DOIs
Publication statusPublished - 15 Mar 2018

Keywords

  • Hole blocking layer
  • Magnetron sputtering
  • Perovskite solar cell
  • Room temperature
  • SnO

ASJC Scopus subject areas

  • General Chemistry
  • Condensed Matter Physics
  • General Physics and Astronomy
  • Surfaces and Interfaces
  • Surfaces, Coatings and Films

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