Numerical and experimental studies on the fracture behavior of rubber-toughened epoxy in bulk specimen and laminated composites

To study the toughening mechanisms of liquid rubber (LR) and core-shell rubber (CSR) in bulk epoxy and composite laminate, experimental and numerical investigations were carried out on compact tension (CT) and double-cantilever-beam (DCB) specimens under mode-I loading. The matrix materials were pure epoxy (DGEBA), 15% LR (CTBN) and 15% CSR modified epoxies. Experimental results and numerical analyses showed that both liquid rubber (LR) and core-shell rubber (CSR) could improve significantly the fracture toughness of pure epoxy (DGEBA). However, the high toughness of these toughened epoxies could not be completely transferred to the interlaminar fracture toughness of the unidirectional carbon fibre reinforced laminate. The main toughening mechanism of CSR in bulk epoxy was the extensive particle cavitation, which greatly released the crack-tip triaxiality and promoted matrix shear plasticity. The poor toughness behavior of CSR in the carbon fibre laminate was thought to be caused by the high constraint imposed by the stiff fibre layers. No particle cavitation had been observed in LR modified epoxy and the main toughening mechanism was merely the large plastic deformation near the crack-tip due to the rubber domains in the matrix which results in a lower yield strength but a higher elongation-to-break.