Influence of Plasmonic Effect on the Upconversion Emission Characteristics of NaYF4 Hexagonal Microrods

Ting Wang; Chun Kit Siu; Huan Yu; Yunfeng Wang; Siqi Li; Wei Lu; Jianhua Hao; Hong Liu; Jing Hua Teng; Dang Yuan Lei; Xuhui Xu; Siu Fung Yu

doi:10.1021/acs.inorgchem.8b00690

Influence of Plasmonic Effect on the Upconversion Emission Characteristics of NaYF₄ Hexagonal Microrods

Ting Wang, Chun Kit Siu, Huan Yu, Yunfeng Wang, Siqi Li, Wei Lu, Jianhua Hao, Hong Liu, Jing Hua Teng, Dang Yuan Lei, Xuhui Xu, Siu Fung Yu

Research output: Journal article publication › Journal article › Academic research › peer-review

20 Citations (Scopus)

Abstract

The influence of plasmonic effect on the upconversion emission characteristics of Yb³⁺-Er³⁺-Tm³⁺ tridoped β-NaYF₄ hexagonal microrods is studied. Upconversion spontaneous emission can be improved by 10 times if the microrod is deposited on an Ag-coated substrate. The enhancement is also dependent on the emission wavelength and the polarization of the excitation source. Furthermore, upconversion lasing is supported by the geometry of the microrods via the formation of whispering gallery modes. The corresponding excitation threshold can also be reduced by 50% through the influence of plasmonic effect, the coupling between the whispering gallery modes and the surface plasmonic resonance modes.

Original language	English
Pages (from-to)	8200-8204
Number of pages	5
Journal	Inorganic Chemistry
Volume	57
Issue number	14
DOIs	https://doi.org/10.1021/acs.inorgchem.8b00690
Publication status	Published - 16 Jul 2018

ASJC Scopus subject areas

Physical and Theoretical Chemistry
Inorganic Chemistry

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10.1021/acs.inorgchem.8b00690

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title = "Influence of Plasmonic Effect on the Upconversion Emission Characteristics of NaYF4 Hexagonal Microrods",

abstract = "The influence of plasmonic effect on the upconversion emission characteristics of Yb3+-Er3+-Tm3+ tridoped β-NaYF4 hexagonal microrods is studied. Upconversion spontaneous emission can be improved by 10 times if the microrod is deposited on an Ag-coated substrate. The enhancement is also dependent on the emission wavelength and the polarization of the excitation source. Furthermore, upconversion lasing is supported by the geometry of the microrods via the formation of whispering gallery modes. The corresponding excitation threshold can also be reduced by 50% through the influence of plasmonic effect, the coupling between the whispering gallery modes and the surface plasmonic resonance modes.",

author = "Ting Wang and Siu, {Chun Kit} and Huan Yu and Yunfeng Wang and Siqi Li and Wei Lu and Jianhua Hao and Hong Liu and Teng, {Jing Hua} and Lei, {Dang Yuan} and Xuhui Xu and Yu, {Siu Fung}",

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T1 - Influence of Plasmonic Effect on the Upconversion Emission Characteristics of NaYF4 Hexagonal Microrods

AU - Wang, Ting

AU - Siu, Chun Kit

AU - Yu, Huan

AU - Wang, Yunfeng

AU - Li, Siqi

AU - Lu, Wei

AU - Hao, Jianhua

AU - Liu, Hong

AU - Teng, Jing Hua

AU - Lei, Dang Yuan

AU - Xu, Xuhui

AU - Yu, Siu Fung

PY - 2018/7/16

Y1 - 2018/7/16

N2 - The influence of plasmonic effect on the upconversion emission characteristics of Yb3+-Er3+-Tm3+ tridoped β-NaYF4 hexagonal microrods is studied. Upconversion spontaneous emission can be improved by 10 times if the microrod is deposited on an Ag-coated substrate. The enhancement is also dependent on the emission wavelength and the polarization of the excitation source. Furthermore, upconversion lasing is supported by the geometry of the microrods via the formation of whispering gallery modes. The corresponding excitation threshold can also be reduced by 50% through the influence of plasmonic effect, the coupling between the whispering gallery modes and the surface plasmonic resonance modes.

AB - The influence of plasmonic effect on the upconversion emission characteristics of Yb3+-Er3+-Tm3+ tridoped β-NaYF4 hexagonal microrods is studied. Upconversion spontaneous emission can be improved by 10 times if the microrod is deposited on an Ag-coated substrate. The enhancement is also dependent on the emission wavelength and the polarization of the excitation source. Furthermore, upconversion lasing is supported by the geometry of the microrods via the formation of whispering gallery modes. The corresponding excitation threshold can also be reduced by 50% through the influence of plasmonic effect, the coupling between the whispering gallery modes and the surface plasmonic resonance modes.

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DO - 10.1021/acs.inorgchem.8b00690

M3 - Journal article

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SN - 0020-1669

VL - 57

SP - 8200

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JO - Inorganic Chemistry

JF - Inorganic Chemistry

IS - 14

ER -

Influence of Plasmonic Effect on the Upconversion Emission Characteristics of NaYF₄ Hexagonal Microrods

Abstract

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