High-Performance Copper-Doped Perovskite-Related Silver Halide X-ray Imaging Scintillator

Tengyue He, Yang Zhou, Xiaojia Wang, Jun Yin, Luis Gutiérrez-Arzaluz, Jian Xin Wang, Yuhai Zhang, Osman M. Bakr, Omar F. Mohammed

Research output: Journal article publicationJournal articleAcademic researchpeer-review

66 Citations (Scopus)

Abstract

Scintillators are critical for high-energy radiation detection across a wide array of potential applications, from medical radiography and safety inspections all the way to space exploration. However, constrained by their current shortcomings, including high-temperature and complex fabrication as well as inherent brittleness and fragility among thick films and bulk crystals, traditional scintillators are finding it difficult to meet the rising demand for cost-effective, ecofriendly, and flexible X-ray detection. Here, we describe the development of high-performance and flexible X-ray scintillators based on films of Cu-doped Cs2AgI3that exhibit ultrahigh X-ray sensitivity. The materials exhibit a high scintillation light yield of up to 82 900 photons/MeV and a low detection limit of 77.8 nGy/s, which is approximately 70 times lower than the dosage for a standard medical examination. Moreover, richly detailed X-ray images of biological tissue and electronic components with a high spatial resolution of 16.2 lp/mm were obtained using flexible, large-area, solution-processed scintillation screens.

Original languageEnglish
Pages (from-to)2753-2760
Number of pages8
JournalACS Energy Letters
Volume7
Issue number8
DOIs
Publication statusPublished - 26 Jul 2022

ASJC Scopus subject areas

  • Chemistry (miscellaneous)
  • Renewable Energy, Sustainability and the Environment
  • Fuel Technology
  • Energy Engineering and Power Technology
  • Materials Chemistry

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