Giant and tunable optical nonlinearity in single-crystalline 2D perovskites due to excitonic and plasma effects

Paul Dichtl; Ibrahim Abdelwahab; Gustavo Grinblat; Kai Leng; Xiao Chi; In Hyeok Park; Michael P. Nielsen; Rupert F. Oulton; Kian Ping Loh; Stefan A. Maier

doi:10.1364/FIO.2019.FTu5F.3

Giant and tunable optical nonlinearity in single-crystalline 2D perovskites due to excitonic and plasma effects

Paul Dichtl
, Ibrahim Abdelwahab
, Gustavo Grinblat
, Kai Leng
, Xiao Chi
, In Hyeok Park
, Michael P. Nielsen
, Rupert F. Oulton
, Kian Ping Loh
, Stefan A. Maier

Research output: Chapter in book / Conference proceeding › Conference article published in proceeding or book › Academic research › peer-review

Abstract

2D Ruddlesden-Popper-type lead halide perovskites exhibit a strong third-order nonlinear response around excitonic resonance, which is characterized with Z-scan measurements. We find large absolute values and a sign change of both nonlinear refraction and absorption.

Original language	English
Title of host publication	Frontiers in Optics - Proceedings Frontiers in Optics + Laser Science APS/DLS
Publisher	Optical Society of America (OSA)
ISBN (Electronic)	9781943580675
DOIs	https://doi.org/10.1364/FIO.2019.FTu5F.3
Publication status	Published - 8 Sept 2019
Externally published	Yes
Event	Frontiers in Optics, FIO 2019 - Part of Frontiers in Optics + Laser Science APS/DLS - Washington, United States Duration: 15 Sept 2019 → 19 Sept 2019

Publication series

Name	Frontiers in Optics - Proceedings Frontiers in Optics + Laser Science APS/DLS

Conference

Conference	Frontiers in Optics, FIO 2019 - Part of Frontiers in Optics + Laser Science APS/DLS
Country/Territory	United States
City	Washington
Period	15/09/19 → 19/09/19

ASJC Scopus subject areas

Atomic and Molecular Physics, and Optics

More information

10.1364/FIO.2019.FTu5F.3

Cite this

Dichtl, P., Abdelwahab, I., Grinblat, G., Leng, K., Chi, X., Park, I. H., Nielsen, M. P., Oulton, R. F., Loh, K. P., & Maier, S. A. (2019). Giant and tunable optical nonlinearity in single-crystalline 2D perovskites due to excitonic and plasma effects. In Frontiers in Optics - Proceedings Frontiers in Optics + Laser Science APS/DLS Article FTu5F.3 (Frontiers in Optics - Proceedings Frontiers in Optics + Laser Science APS/DLS). Optical Society of America (OSA). https://doi.org/10.1364/FIO.2019.FTu5F.3

Dichtl, Paul ; Abdelwahab, Ibrahim ; Grinblat, Gustavo et al. / Giant and tunable optical nonlinearity in single-crystalline 2D perovskites due to excitonic and plasma effects. Frontiers in Optics - Proceedings Frontiers in Optics + Laser Science APS/DLS. Optical Society of America (OSA), 2019. (Frontiers in Optics - Proceedings Frontiers in Optics + Laser Science APS/DLS).

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title = "Giant and tunable optical nonlinearity in single-crystalline 2D perovskites due to excitonic and plasma effects",

abstract = "2D Ruddlesden-Popper-type lead halide perovskites exhibit a strong third-order nonlinear response around excitonic resonance, which is characterized with Z-scan measurements. We find large absolute values and a sign change of both nonlinear refraction and absorption.",

author = "Paul Dichtl and Ibrahim Abdelwahab and Gustavo Grinblat and Kai Leng and Xiao Chi and Park, \{In Hyeok\} and Nielsen, \{Michael P.\} and Oulton, \{Rupert F.\} and Loh, \{Kian Ping\} and Maier, \{Stefan A.\}",

note = "Publisher Copyright: {\textcopyright} OSA 2019. The Author(s).; Frontiers in Optics, FIO 2019 - Part of Frontiers in Optics + Laser Science APS/DLS ; Conference date: 15-09-2019 Through 19-09-2019",

year = "2019",

month = sep,

day = "8",

doi = "10.1364/FIO.2019.FTu5F.3",

language = "English",

series = "Frontiers in Optics - Proceedings Frontiers in Optics + Laser Science APS/DLS",

publisher = "Optical Society of America (OSA)",

booktitle = "Frontiers in Optics - Proceedings Frontiers in Optics + Laser Science APS/DLS",

}

Dichtl, P, Abdelwahab, I, Grinblat, G, Leng, K, Chi, X, Park, IH, Nielsen, MP, Oulton, RF, Loh, KP & Maier, SA 2019, Giant and tunable optical nonlinearity in single-crystalline 2D perovskites due to excitonic and plasma effects. in Frontiers in Optics - Proceedings Frontiers in Optics + Laser Science APS/DLS., FTu5F.3, Frontiers in Optics - Proceedings Frontiers in Optics + Laser Science APS/DLS, Optical Society of America (OSA), Frontiers in Optics, FIO 2019 - Part of Frontiers in Optics + Laser Science APS/DLS, Washington, United States, 15/09/19. https://doi.org/10.1364/FIO.2019.FTu5F.3

Giant and tunable optical nonlinearity in single-crystalline 2D perovskites due to excitonic and plasma effects. / Dichtl, Paul; Abdelwahab, Ibrahim; Grinblat, Gustavo et al.
Frontiers in Optics - Proceedings Frontiers in Optics + Laser Science APS/DLS. Optical Society of America (OSA), 2019. FTu5F.3 (Frontiers in Optics - Proceedings Frontiers in Optics + Laser Science APS/DLS).

Research output: Chapter in book / Conference proceeding › Conference article published in proceeding or book › Academic research › peer-review

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AU - Dichtl, Paul

AU - Abdelwahab, Ibrahim

AU - Grinblat, Gustavo

AU - Leng, Kai

AU - Chi, Xiao

AU - Park, In Hyeok

AU - Nielsen, Michael P.

AU - Oulton, Rupert F.

AU - Loh, Kian Ping

AU - Maier, Stefan A.

PY - 2019/9/8

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AB - 2D Ruddlesden-Popper-type lead halide perovskites exhibit a strong third-order nonlinear response around excitonic resonance, which is characterized with Z-scan measurements. We find large absolute values and a sign change of both nonlinear refraction and absorption.

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DO - 10.1364/FIO.2019.FTu5F.3

M3 - Conference article published in proceeding or book

AN - SCOPUS:85087107144

T3 - Frontiers in Optics - Proceedings Frontiers in Optics + Laser Science APS/DLS

BT - Frontiers in Optics - Proceedings Frontiers in Optics + Laser Science APS/DLS

PB - Optical Society of America (OSA)

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Dichtl P, Abdelwahab I, Grinblat G, Leng K, Chi X, Park IH et al. Giant and tunable optical nonlinearity in single-crystalline 2D perovskites due to excitonic and plasma effects. In Frontiers in Optics - Proceedings Frontiers in Optics + Laser Science APS/DLS. Optical Society of America (OSA). 2019. FTu5F.3. (Frontiers in Optics - Proceedings Frontiers in Optics + Laser Science APS/DLS). doi: 10.1364/FIO.2019.FTu5F.3

Giant and tunable optical nonlinearity in single-crystalline 2D perovskites due to excitonic and plasma effects

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