Giant and tunable optical nonlinearity in single-crystalline 2D perovskites due to excitonic and plasma effects

Paul Dichtl; Ibrahim Abdelwahab; Gustavo Grinblat; Kai Leng; Xiao Chi; In Hyeok Park; Michael P. Nielsen; Rupert F. Oulton; Kian Ping Loh; Stefan A. Maier

doi:10.1364/FIO.2019.FTu5F.3

Giant and tunable optical nonlinearity in single-crystalline 2D perovskites due to excitonic and plasma effects

Paul Dichtl, Ibrahim Abdelwahab, Gustavo Grinblat, Kai Leng, Xiao Chi, In Hyeok Park, Michael P. Nielsen, Rupert F. Oulton, Kian Ping Loh, Stefan A. Maier

Research output: Chapter in book / Conference proceeding › Conference article published in proceeding or book › Academic research › peer-review

Abstract

2D Ruddlesden-Popper-type lead halide perovskites exhibit a strong third-order nonlinear response around excitonic resonance, which is characterized with Z-scan measurements. We find large absolute values and a sign change of both nonlinear refraction and absorption.

Original language	English
Title of host publication	Frontiers in Optics - Proceedings Frontiers in Optics + Laser Science APS/DLS
Publisher	Optical Society of America (OSA)
ISBN (Electronic)	9781943580675
DOIs	https://doi.org/10.1364/FIO.2019.FTu5F.3
Publication status	Published - 8 Sept 2019
Externally published	Yes
Event	Frontiers in Optics, FIO 2019 - Part of Frontiers in Optics + Laser Science APS/DLS - Washington, United States Duration: 15 Sept 2019 → 19 Sept 2019

Publication series

Name	Frontiers in Optics - Proceedings Frontiers in Optics + Laser Science APS/DLS

Conference

Conference	Frontiers in Optics, FIO 2019 - Part of Frontiers in Optics + Laser Science APS/DLS
Country/Territory	United States
City	Washington
Period	15/09/19 → 19/09/19

ASJC Scopus subject areas

Atomic and Molecular Physics, and Optics

More information

10.1364/FIO.2019.FTu5F.3

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Dichtl, P., Abdelwahab, I., Grinblat, G., Leng, K., Chi, X., Park, I. H., Nielsen, M. P., Oulton, R. F., Loh, K. P., & Maier, S. A. (2019). Giant and tunable optical nonlinearity in single-crystalline 2D perovskites due to excitonic and plasma effects. In Frontiers in Optics - Proceedings Frontiers in Optics + Laser Science APS/DLS Article FTu5F.3 (Frontiers in Optics - Proceedings Frontiers in Optics + Laser Science APS/DLS). Optical Society of America (OSA). https://doi.org/10.1364/FIO.2019.FTu5F.3

Dichtl, Paul ; Abdelwahab, Ibrahim ; Grinblat, Gustavo et al. / Giant and tunable optical nonlinearity in single-crystalline 2D perovskites due to excitonic and plasma effects. Frontiers in Optics - Proceedings Frontiers in Optics + Laser Science APS/DLS. Optical Society of America (OSA), 2019. (Frontiers in Optics - Proceedings Frontiers in Optics + Laser Science APS/DLS).

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title = "Giant and tunable optical nonlinearity in single-crystalline 2D perovskites due to excitonic and plasma effects",

abstract = "2D Ruddlesden-Popper-type lead halide perovskites exhibit a strong third-order nonlinear response around excitonic resonance, which is characterized with Z-scan measurements. We find large absolute values and a sign change of both nonlinear refraction and absorption.",

author = "Paul Dichtl and Ibrahim Abdelwahab and Gustavo Grinblat and Kai Leng and Xiao Chi and Park, {In Hyeok} and Nielsen, {Michael P.} and Oulton, {Rupert F.} and Loh, {Kian Ping} and Maier, {Stefan A.}",

note = "Publisher Copyright: {\textcopyright} OSA 2019. The Author(s).; Frontiers in Optics, FIO 2019 - Part of Frontiers in Optics + Laser Science APS/DLS ; Conference date: 15-09-2019 Through 19-09-2019",

year = "2019",

month = sep,

day = "8",

doi = "10.1364/FIO.2019.FTu5F.3",

language = "English",

series = "Frontiers in Optics - Proceedings Frontiers in Optics + Laser Science APS/DLS",

publisher = "Optical Society of America (OSA)",

booktitle = "Frontiers in Optics - Proceedings Frontiers in Optics + Laser Science APS/DLS",

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Dichtl, P, Abdelwahab, I, Grinblat, G, Leng, K, Chi, X, Park, IH, Nielsen, MP, Oulton, RF, Loh, KP & Maier, SA 2019, Giant and tunable optical nonlinearity in single-crystalline 2D perovskites due to excitonic and plasma effects. in Frontiers in Optics - Proceedings Frontiers in Optics + Laser Science APS/DLS., FTu5F.3, Frontiers in Optics - Proceedings Frontiers in Optics + Laser Science APS/DLS, Optical Society of America (OSA), Frontiers in Optics, FIO 2019 - Part of Frontiers in Optics + Laser Science APS/DLS, Washington, United States, 15/09/19. https://doi.org/10.1364/FIO.2019.FTu5F.3

Giant and tunable optical nonlinearity in single-crystalline 2D perovskites due to excitonic and plasma effects. / Dichtl, Paul; Abdelwahab, Ibrahim; Grinblat, Gustavo et al.
Frontiers in Optics - Proceedings Frontiers in Optics + Laser Science APS/DLS. Optical Society of America (OSA), 2019. FTu5F.3 (Frontiers in Optics - Proceedings Frontiers in Optics + Laser Science APS/DLS).

Research output: Chapter in book / Conference proceeding › Conference article published in proceeding or book › Academic research › peer-review

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AU - Dichtl, Paul

AU - Abdelwahab, Ibrahim

AU - Grinblat, Gustavo

AU - Leng, Kai

AU - Chi, Xiao

AU - Park, In Hyeok

AU - Nielsen, Michael P.

AU - Oulton, Rupert F.

AU - Loh, Kian Ping

AU - Maier, Stefan A.

PY - 2019/9/8

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AB - 2D Ruddlesden-Popper-type lead halide perovskites exhibit a strong third-order nonlinear response around excitonic resonance, which is characterized with Z-scan measurements. We find large absolute values and a sign change of both nonlinear refraction and absorption.

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T3 - Frontiers in Optics - Proceedings Frontiers in Optics + Laser Science APS/DLS

BT - Frontiers in Optics - Proceedings Frontiers in Optics + Laser Science APS/DLS

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Dichtl P, Abdelwahab I, Grinblat G, Leng K, Chi X, Park IH et al. Giant and tunable optical nonlinearity in single-crystalline 2D perovskites due to excitonic and plasma effects. In Frontiers in Optics - Proceedings Frontiers in Optics + Laser Science APS/DLS. Optical Society of America (OSA). 2019. FTu5F.3. (Frontiers in Optics - Proceedings Frontiers in Optics + Laser Science APS/DLS). doi: 10.1364/FIO.2019.FTu5F.3

Giant and tunable optical nonlinearity in single-crystalline 2D perovskites due to excitonic and plasma effects

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