Effects of Sea Salt Aerosol Emissions for Marine Cloud Brightening on Atmospheric Chemistry: Implications for Radiative Forcing

Hannah M. Horowitz, Christopher Holmes, Alicia Wright, Tomás Sherwen, Xuan Wang, Mat Evans, Jiayue Huang, Lyatt Jaeglé, Qianjie Chen, Shuting Zhai, Becky Alexander

Research output: Journal article publicationJournal articleAcademic researchpeer-review

1 Citation (Scopus)

Abstract

Marine cloud brightening (MCB) is proposed to offset global warming by emitting sea salt aerosols to the tropical marine boundary layer, which increases aerosol and cloud albedo. Sea salt aerosol is the main source of tropospheric reactive chlorine (Cly) and bromine (Bry). The effects of additional sea salt on atmospheric chemistry have not been explored. We simulate sea salt aerosol injections for MCB under two scenarios (212–569 Tg/a) in the GEOS-Chem global chemical transport model, only considering their impacts as a halogen source. Globally, tropospheric Cly and Bry increase (20–40%), leading to decreased ozone (−3 to −6%). Consequently, OH decreases (−3 to −5%), which increases the methane lifetime (3–6%). Our results suggest that the chemistry of the additional sea salt leads to minor total radiative forcing compared to that of the sea salt aerosol itself (~2%) but may have potential implications for surface ozone pollution in tropical coastal regions.

Original languageEnglish
Article numbere2019GL085838
JournalGeophysical Research Letters
Volume47
Issue number4
DOIs
Publication statusPublished - 28 Feb 2020
Externally publishedYes

Keywords

  • atmospheric chemistry
  • geoengineering
  • marine cloud brightening
  • reactive halogens
  • sea salt aerosols

ASJC Scopus subject areas

  • Geophysics
  • Earth and Planetary Sciences(all)

Cite this