Cryogenic dielectric and piezoelectric activities in rhombohedral (1 - X)Pb(Mg1/3Nb2/3)O3-xPbTiO3single crystals with different crystallographic orientations

Feifei Wang, Siu Wing Or, Xiangyong Zhao, Haosu Luo

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16 Citations (Scopus)


We report the cryogenic dielectric and piezoelectric activities in [0 0 1]-, [1 1 0]- and [1 1 1]-oriented rhombohedral (1 - x)Pb(Mg1/3Nb2/3)O3-xPbTiO3single crystals for temperatures down to -200 °C. Unusual dielectric relaxation resulting from collective pinning of randomly distributed point defects to ferroelectric macrodomain walls is observed instead of a phase transition in all the poled crystals below -150 °C rather than in the unpoled ones. Stiffening of the poled crystals by the cryogenic temperature-induced pinning effect leads to a characteristic decrease in the piezoelectric coefficient (d31) and the compliance coefficient ( ), along with a similar quantitative increase in frequency constant (N31). An almost temperature-independent property region is revealed in a wide temperature range of -50 to -150 °C, enabling applications of the crystals in cryogenic fields.
Original languageEnglish
Article number182001
JournalJournal of Physics D: Applied Physics
Issue number18
Publication statusPublished - 17 Sep 2009

ASJC Scopus subject areas

  • Electronic, Optical and Magnetic Materials
  • Condensed Matter Physics
  • Acoustics and Ultrasonics
  • Surfaces, Coatings and Films

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