Achieving efficient green-solvent-processed organic solar cells by employing ortho-ortho perylene diimide dimer

Helin Wang, Jiatao Wu, Youming Zhang, Jun Song, Lingcheng Chen, Yi Xiao, Junle Qu, Wai Yeung Wong (Corresponding Author)

Research output: Journal article publicationJournal articleAcademic researchpeer-review

4 Citations (Scopus)

Abstract

The lack of electron acceptors with suitable green solvent processing and excellent device performance is an important problem that hinders the development and commercialization of organic solar cells (OSCs). Here, an ortho-ortho perylene diimide (PDI) dimer (oo-2PDI) is developed and used as an acceptor for use in efficient green-solvent-processed (GSP) OSCs. By using chlorobenzene (CB), anisole, and ortho-xylene as the processing solvents, power conversion efficiencies (PCEs) of 5.04%, 5.03%, and 5.78% were achieved without the additive, respectively. In addition, the non-fullerene oo-2PDI-based GSPOSCs show superior photovoltaic performance to [6,6]-phenyl-C61-butyric acid methyl ester (PCBM)-based GSPOSCs under identical conditions. Therefore, these results demonstrate the possibility of achieving efficient non-fullerene GSPOSCs.

Original languageEnglish
Article number105732
JournalOrganic Electronics
Volume83
DOIs
Publication statusPublished - Aug 2020

Keywords

  • Electron acceptor
  • Green solvent
  • Organic solar cell
  • Ortho-ortho dimer
  • Perylene diimide

ASJC Scopus subject areas

  • Electronic, Optical and Magnetic Materials
  • Biomaterials
  • Chemistry(all)
  • Condensed Matter Physics
  • Materials Chemistry
  • Electrical and Electronic Engineering

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