2H-MoS2 lubrication-enhanced MWCNT nanocomposite for subtle bio-motion piezoresistive detection with deep learning integration

Ke Yu Yao, Derek Ka Hei Lai, Hyo Jung Lim, Bryan Pak Hei So, Andy Chi Ho Chan, Patrick Yiu Man Yip, Duo Wai Chi Wong, Bingyang Dai, Xin Zhao, Siu Hong Dexter Wong, James Chung Wai Cheung

Research output: Journal article publicationJournal articleAcademic researchpeer-review

Abstract

Intelligent piezoresistive health monitoring systems integrate advanced nanocomposite architectures with precise algorithmic analysis for real-time physiological assessment. However, existing works often prioritize high sensitivity at the expense of strain tolerance and require complex fabrication procedures. Herein, we present an environmentally friendly, low-cost, and nonionic fabrication approach for a 2H-phase molybdenum disulfide (2H-MoS2)-enhanced multi-walled carbon nanotube (MWCNT) strain sensor, developed via a systematically optimized vacuum-assisted filtration process. This study is the first to validate the dual enhancement effect of MoS2, leveraging its shear-exfoliation properties to simultaneously improve strain gauge performance and mechanical robustness. The resulting nacre-like layered hybrid nanocomposite achieves a remarkable gauge factor of 675.7 (R2∼0.993) at low strain (∼0–4.5 %), representing a 3881.5 % improvement over pure MWCNT systems, alongside enhanced toughness (∼89.17 %) and strain tolerance (∼53.93 %). Meanwhile, the optimized composition ensures low rest-state resistance (∼13.1 Ω), minimal hysteresis (∼5.7 %), and robust durability over 5000 cycles at 10 % strain. As a result, the proposed sensor enables highly consistent, high-fidelity monitoring of various subtle-to-moderate biomotions. Integrated with a fine-tuned InceptionTime deep learning model, it achieves an F1-score of 98 % in classifying Dysphagia Diet Standardization Initiative (IDDSI)-standard swallowing activities, demonstrating its potential for AI-driven health monitoring applications.

Original languageEnglish
Article number113861
JournalMaterials and Design
Volume253
DOIs
Publication statusPublished - May 2025

Keywords

  • Deep learning
  • Flexible piezoresistive sensor
  • Lubrication toughening
  • MWCNT/MoS nanocomposite
  • Subtle-to-moderate biophysical signal

ASJC Scopus subject areas

  • General Materials Science
  • Mechanics of Materials
  • Mechanical Engineering

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